作者:Hu, Shuaifeng; Wang, Junke; Zhao, Pei; Pascual, Jorge; Wang, Jianan; Rombach, Florine; Dasgupta, Akash; Liu, Wentao; Truong, Minh Anh; Zhu, He; Kober-Czerny, Manuel; Drysdale, James N.; Smith, Joel A.; Yuan, Zhongcheng; Aalbers, Guus J. W.; Schipper, Nick R. M.; Yao, Jin; Nakano, Kyohei; Turren-Cruz, Silver-Hamill; Dallmann, Andre; Christoforo, M. Greyson; Ball, James M.; Mcmeekin, David P.; Zaininger, Karl-Augustin; Liu, Zonghao; Noel, Nakita K.; Tajima, Keisuke; Chen, Wei; Ehara, Masahiro; Janssen, Rene A. J.; Wakamiya, Atsushi; Snaith, Henry J.
作者单位:University of Oxford; Kyoto University; National Institutes of Natural Sciences (NINS) - Japan; Institute for Molecular Science (IMS); University of Basque Country; POLYMAT; Huazhong University of Science & Technology; Eindhoven University of Technology; Eindhoven University of Technology; University of Oxford; RIKEN; University of Valencia; Humboldt University of Berlin
摘要:Multijunction photovoltaics (PVs) are gaining prominence owing to their superior capability of achieving power conversion efficiencies (PCEs) beyond the radiative limit of single-junction cells1, 2, 3, 4, 5, 6, 7-8, for which improving narrow-bandgap (NBG) tin-lead perovskites is critical for thin-film devices9. Here, with a focus on understanding the chemistry of tin-lead perovskite precursor solutions, we find that Sn(ii) species dominate interactions with precursors and additives and uncove...