Controlling laser-dressed resonance line shape using attosecond extreme-ultraviolet pulse with a spectral minimum

• 成果类型: Article
• 署名作者: Fu, Yong; Wang, Bincheng; Wang, Kan; Tang, Xiangyu; Li, Baochang; Yin, Zhiming; Han, Jiaxin; Lin, C. D.; Jin, Cheng
• 署名单位: Nanjing University of Science & Technology; Kansas State University; Nanjing University of Science & Technology
• 刊物名称: PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
• ISSN/ISSBN: 0027-12155
• DOI: 10.1073/pnas.2307836121
• 发表日期: 2024-01-09
• 关键词: fano resonance; phase

摘要

High-harmonic generation from a gas target exhibits sharp spectral features and rapid phase variation near the Cooper minimum. By applying spectral filtering, shaped isolated attosecond pulses can be generated where the pulse is split into two in the time domain. Using such shaped extreme-ultraviolet (XUV) pulses, we theoretically study attosecond transient absorption (ATA) spectra of helium 2s2p autoionizing state which is resonantly coupled to the 2s2 dark state by a time-delayed infrared laser. Our simulations show that the asymmetric 2s2p Fano line shape can be readily tuned into symmetric Lorentzian within the time delay of a few tens of attoseconds. Such efficient control is due to the destructive interference in the generation of the 2s2p state when it is excited by a strongly shaped XUV pulse. This is to be compared to prior experiments where tuning the line shape of a Fano resonance would take tens of femtoseconds. We also show that the predicted ATA spectral line shape can be observed experimentally after propagation in a gas medium. Our results suggest that strongly shaped attosecond XUV pulses offer the opportunity for controlling and probing fine features of narrow resonances on the few-ten attoseconds timescale.