Trends in the seasonal amplitude of atmospheric methane

• 成果类型: Article
• 署名作者: Liu, Gang; Shen, Lu; Ciais, Philippe; Lin, Xin; Hauglustaine, Didier; Lan, Xin; Turner, Alexander J.; Xi, Yi; Zhu, Yu; Peng, Shushi
• 署名单位: Peking University; Peking University; Peking University; CEA; Universite Paris Saclay; University of Colorado System; University of Colorado Boulder; National Oceanic Atmospheric Admin (NOAA) - USA; University of Washington; University of Washington Seattle
• 刊物名称: Nature
• ISSN/ISSBN: 0028-1607
• DOI: 10.1038/s41586-025-08900-8
• 发表日期: 2025-05-15
• 关键词: high-latitudes; emissions; co2; models; GROWTH; constraints; satellite; chemistry; aerosols; orchidee

摘要

Methane is an important greenhouse gas1 and its atmospheric concentration has almost tripled since pre-industrial times2, 3-4. Atmospheric methane mixing ratios vary seasonally, with the seasonal cycle amplitude (SCA) having decreased in northern high latitudes and increased in the subtropics and tropics since the 1980s5,6. These opposing SCA trends can help understanding of long-term changes in the global methane budget, as methane emissions and sinks have opposing effects on the SCA5. However, trends in the methane SCA have not yet been explored in detail5,6. Here we use a suite of atmospheric transport model simulations and attribute the observed trends in the seasonal amplitude of methane to changes in emissions and the atmospheric sink from reaction with the hydroxyl radical (OH). We find that the decreasing amplitude in the northern high latitudes is mainly caused by an increase in natural emissions (such as wetlands) owing to a warmer climate, adding evidence to previous studies suggesting a positive climate feedback7, 8-9. In contrast, the enhanced methane amplitude in the subtropics and tropics is mainly attributed to strengthened OH oxidation. Our results provide independent evidence for an increase in tropospheric OH concentration10,11 of 10 +/- 1% since 1984, which together with an increasing atmospheric methane concentration suggests a 21 +/- 1% increase in the atmospheric methane sink.