Vertically stacked monolithic perovskite colour photodetectors
成果类型：
Article
署名作者：
Tsarev, Sergey; Proniakova, Daria; Liu, Xuqi; Wu, Erfu; Matt, Gebhard J.; Sakhatskyi, Kostiantyn; Ferraresi, Lorenzo L. A.; Kothandaraman, Radha; Fu, Fan; Shorubalko, Ivan; Yakunin, Sergii; Kovalenko, Maksym V.
署名单位：
Swiss Federal Institutes of Technology Domain; ETH Zurich; Swiss Federal Institutes of Technology Domain; Swiss Federal Laboratories for Materials Science & Technology (EMPA); Swiss Federal Institutes of Technology Domain; Swiss Federal Laboratories for Materials Science & Technology (EMPA)
刊物名称：
Nature
ISSN/ISSBN：
0028-1515
DOI：
10.1038/s41586-025-09062-3
发表日期：
2025-06-19
关键词：
efficient
摘要：
Modern colour image sensors face challenges in further improving sensitivity and image quality because of inherent limitations in light utilization efficiency1. A major factor contributing to these limitations is the use of passive optical filters, which absorb and dissipate a substantial amount of light, thereby reducing the efficiency of light capture2. On the contrary, active optical filtering in Foveon-type vertically stacked architectures still struggles to deliver optimal performance owing to their lack of colour selectivity, making them inefficient for precise colour imaging3. Here we introduce an innovative architecture for colour sensor arrays that uses multilayer monolithically stacked lead halide perovskite thin-film photodetectors. Perovskite bandgap tunability4 is utilized to selectively absorb the visible light spectrum's red, green and blue regions, eliminating the need for colour filters. External quantum efficiencies of 50%, 47% and 53% are demonstrated for the red, green and blue channels, respectively, as well as a colour accuracy of 3.8% in Delta ELab outperforming the state-of-the-art colour-filter array and Foveon-type photosensors. The image sensor design improves light utilization in colour sensors and paves the way for the next generation of highly sensitive, artefact-free images with enhanced colour fidelity.